I went for 46:22 with a 113T tooth belt. I could never quote get enough tnesion, so when I had new dropouts made to use the bolt-in hub, I tweaked the geometry to get an extra 3mm.
I’m going to replace it with 46:24 so I can bring the back wheel in, and actually get up steep hills without risking over-torquing the belt, which is what killed it.
You have to bear in mind the width if the sprockets, especially the front one. If you go too large, you could get a clash on the chainstay. I dpn’t know if drawings of the Centretrack sprockets are available, I certainly used to have a set for the Carbon-Drive versions.