I’ve had that fork and those pressure seem a little high.
I completely agree with the others thsat say sometimes too low pressure can feel harsh due to hitting the ramp up too early. I’ve had that happen several times on other forks. But I was around 180 lbs and running 80psi in my Rhythm 34 and it felt great, so i think 100 psi might be a little high. I had zero tokens. If installing tokens, generally reduce the psi a little.
I beleive the compression dial is overall compression, not LSC. So by dialling in some compression, unfortunately you are increasing LSC support (less diving = good) but also increasing HSC which I found made it harsh. That’s when I started noticing the limitations to that fork, after having other forks with dedicated LSC/HSC so you could dial in a little LSC support but still keep the HSC wide open to keep it plush.