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BladeRunner for sure, The anime Wings of Honneamise has a beautiful Ryuichi Sakamoto soundtrack, Goodbye Mr Lawrence too.
There was also to be a version of Dune from the mid 70's which would have had an AMAZING soundtrack; Pink Floyd, Tangerine Dream etc.
Dust Brothers - Fight Club
and thought Daft Punk - Tron Legacy was inspired
Human Traffic,
Lock Stock and Two Smoking Barrels,
Highlander,
Oceans Eleven,
Shopping,
Blade Runner,
Trainspotting,
Any Bond film scored by John Barry.
Not sure about 'best of all time' but the Dances with Wolves score is quite beautiful
The Last Temptation of Christ: Peter Gabrials Passion
Platoon :Who will eva forget Barbers Adagio for strings
The Life Aquatic with Steve Zissou :David Bowie in Portugese
FM soundtrack :An early 80's film with a gr8 soundtrack