It is not really a question of material as much as it is a question of construction/builder.
You have to remember that any “standard” commercially available bike or frame is going to be built en masse in a factory and even the best of them suffer from an element of sacrificing design elements to aid building.
If you do want a really good riding experience go for a handbuilt frame ( and by handbuilt I mean just that & not a factory bile that is braised/welded by people ) An experienced framebuilder can make both steel & aluminium feel alive, A really good one will talk to you to find out how you ride and then advise you on the best materials for your needs.